Abnormal anti-Stokes Raman scattering of carbon nanotubes

S L Zhang; H D Li; Z J Shi; K T Yue; J Zi; Z N Gu; X H Wu; Z L Lian; Y Zhan; F M Huang; L X Zhou; Y G Zhang; S Iijima

doi:Artn 035413\rDoi 10.1103/Physrevb.66.035413

Abnormal anti-Stokes Raman scattering of carbon nanotubes

S L Zhang, H D Li, Z J Shi, K T Yue, J Zi, Z N Gu, X H Wu, Z L Lian, Y Zhan, F M Huang, L X Zhou, Y G Zhang, S Iijima

School of Mathematics and Physics

Research output: Contribution to journal › Article › peer-review

25 Citations (Scopus)

Abstract

Abnormal anti-Stokes Raman scattering (AASR) was unambiguously observed in carbon nanotubes (CNT's). In contrast to traditional Raman scattering theory, the absolute value of the Raman frequency of the anti-Stokes peak is not the same as that of the corresponding Stokes peak. It was demonstrated that AASR scattering originates from the unique nanoscale cylindrical structure of CNT's that can be considered naturally as a graphite structure with an intrinsic defect from its rolling. The double-resonance Raman scattering theory was applied to interpret the scattering mechanism of the AASR phenomenon successfully and quantitatively.

Original language	English
Journal	Physical Review B (Condensed Matter)
Volume	66
DOIs	https://doi.org/Artn 035413\rDoi 10.1103/Physrevb.66.035413
Publication status	Published - 2002

Keywords

dependence
graphite
modes
spectra

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Artn 035413\rDoi 10.1103/Physrevb.66.035413

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title = "Abnormal anti-Stokes Raman scattering of carbon nanotubes",

abstract = "Abnormal anti-Stokes Raman scattering (AASR) was unambiguously observed in carbon nanotubes (CNT's). In contrast to traditional Raman scattering theory, the absolute value of the Raman frequency of the anti-Stokes peak is not the same as that of the corresponding Stokes peak. It was demonstrated that AASR scattering originates from the unique nanoscale cylindrical structure of CNT's that can be considered naturally as a graphite structure with an intrinsic defect from its rolling. The double-resonance Raman scattering theory was applied to interpret the scattering mechanism of the AASR phenomenon successfully and quantitatively.",

keywords = "dependence, graphite, modes, spectra",

author = "Zhang, {S L} and Li, {H D} and Shi, {Z J} and Yue, {K T} and J Zi and Gu, {Z N} and Wu, {X H} and Lian, {Z L} and Y Zhan and Huang, {F M} and Zhou, {L X} and Zhang, {Y G} and S Iijima",

year = "2002",

doi = "Artn 035413\rDoi 10.1103/Physrevb.66.035413",

language = "English",

volume = "66",

journal = "Physical Review B (Condensed Matter)",

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TY - JOUR

T1 - Abnormal anti-Stokes Raman scattering of carbon nanotubes

AU - Zhang, S L

AU - Li, H D

AU - Shi, Z J

AU - Yue, K T

AU - Zi, J

AU - Gu, Z N

AU - Wu, X H

AU - Lian, Z L

AU - Zhan, Y

AU - Huang, F M

AU - Zhou, L X

AU - Zhang, Y G

AU - Iijima, S

PY - 2002

Y1 - 2002

N2 - Abnormal anti-Stokes Raman scattering (AASR) was unambiguously observed in carbon nanotubes (CNT's). In contrast to traditional Raman scattering theory, the absolute value of the Raman frequency of the anti-Stokes peak is not the same as that of the corresponding Stokes peak. It was demonstrated that AASR scattering originates from the unique nanoscale cylindrical structure of CNT's that can be considered naturally as a graphite structure with an intrinsic defect from its rolling. The double-resonance Raman scattering theory was applied to interpret the scattering mechanism of the AASR phenomenon successfully and quantitatively.

AB - Abnormal anti-Stokes Raman scattering (AASR) was unambiguously observed in carbon nanotubes (CNT's). In contrast to traditional Raman scattering theory, the absolute value of the Raman frequency of the anti-Stokes peak is not the same as that of the corresponding Stokes peak. It was demonstrated that AASR scattering originates from the unique nanoscale cylindrical structure of CNT's that can be considered naturally as a graphite structure with an intrinsic defect from its rolling. The double-resonance Raman scattering theory was applied to interpret the scattering mechanism of the AASR phenomenon successfully and quantitatively.

KW - dependence

KW - graphite

KW - modes

KW - spectra

U2 - Artn 035413\rDoi 10.1103/Physrevb.66.035413

DO - Artn 035413\rDoi 10.1103/Physrevb.66.035413

M3 - Article

SN - 0163-1829

VL - 66

JO - Physical Review B (Condensed Matter)

JF - Physical Review B (Condensed Matter)

ER -

Abnormal anti-Stokes Raman scattering of carbon nanotubes

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Keywords

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