Co-tape casting fabrication, field assistant sintering
and evaluation of a coke resistant
La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode
supported solid oxide fuel cell

Xiaoming Hao; Dongdong Han; Jiawei Wang; Yajie Liu; David Rooney; Wang Sun; Jinshuo Qiao; Zhenhua Wang; Kening Sun

doi:10.1016/j.ijhydene.2015.07.126

Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode supported solid oxide fuel cell

Xiaoming Hao, Dongdong Han, Jiawei Wang, Yajie Liu, David Rooney, Wang Sun, Jinshuo Qiao, Zhenhua Wang^*, Kening Sun

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

11 Citations (Scopus)

Abstract

The ability to directly utilize hydrocarbons and other renewable liquid fuels is one of the most important issues affecting the large scale deployment of solid oxide fuel cells (SOFCs). Herein we designed La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode (FGA) supported SOFCs, prepared with a co-tape casting method and sintered using the field assisted sintering technique (FAST). Through SEM observations, it was confirmed that the FGA structure was achieved and well maintained after the FAST process. Distortion and delamination which usually results after conventional sintering was successfully avoided. The La_0.2Sr_0.7TiO₃-Ni/YSZ FGA supported SOFCs showed a maximum power density of 600mWcm^-2at 750°C, and was stable for 70h in CH₄. No carbon deposition was detected using Raman spectroscopy. These results confirm the potential coke resistance of La_0.2Sr_0.7TiO₃-Ni/YSZ FGA supported SOFCs.

Original language	English
Pages (from-to)	12790-12797
Number of pages	8
Journal	International Journal of Hydrogen Energy
Volume	40
Issue number	37
Early online date	15 Aug 2015
DOIs	https://doi.org/10.1016/j.ijhydene.2015.07.126
Publication status	Published - 05 Oct 2015

Keywords

Field assisted sintering technique
Lanthanum-doped strontium titanate
Solid oxide fuel cells

ASJC Scopus subject areas

Renewable Energy, Sustainability and the Environment
Fuel Technology
Condensed Matter Physics
Energy Engineering and Power Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1016/j.ijhydene.2015.07.126

Cite this

Hao, X., Han, D., Wang, J., Liu, Y., Rooney, D., Sun, W., Qiao, J., Wang, Z., & Sun, K. (2015). Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode supported solid oxide fuel cell. International Journal of Hydrogen Energy, 40(37), 12790-12797. https://doi.org/10.1016/j.ijhydene.2015.07.126

Hao, Xiaoming ; Han, Dongdong ; Wang, Jiawei ; Liu, Yajie ; Rooney, David ; Sun, Wang ; Qiao, Jinshuo ; Wang, Zhenhua ; Sun, Kening. / Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode supported solid oxide fuel cell. In: International Journal of Hydrogen Energy. 2015 ; Vol. 40, No. 37. pp. 12790-12797.

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title = "Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode supported solid oxide fuel cell",

abstract = "The ability to directly utilize hydrocarbons and other renewable liquid fuels is one of the most important issues affecting the large scale deployment of solid oxide fuel cells (SOFCs). Herein we designed La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode (FGA) supported SOFCs, prepared with a co-tape casting method and sintered using the field assisted sintering technique (FAST). Through SEM observations, it was confirmed that the FGA structure was achieved and well maintained after the FAST process. Distortion and delamination which usually results after conventional sintering was successfully avoided. The La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs showed a maximum power density of 600mWcm-2 at 750°C, and was stable for 70h in CH4. No carbon deposition was detected using Raman spectroscopy. These results confirm the potential coke resistance of La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs.",

keywords = "Field assisted sintering technique, Lanthanum-doped strontium titanate, Solid oxide fuel cells",

author = "Xiaoming Hao and Dongdong Han and Jiawei Wang and Yajie Liu and David Rooney and Wang Sun and Jinshuo Qiao and Zhenhua Wang and Kening Sun",

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Hao, X, Han, D, Wang, J, Liu, Y, Rooney, D, Sun, W, Qiao, J, Wang, Z & Sun, K 2015, 'Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode supported solid oxide fuel cell', International Journal of Hydrogen Energy, vol. 40, no. 37, pp. 12790-12797. https://doi.org/10.1016/j.ijhydene.2015.07.126

Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La_0.2Sr_0.7TiO₃-Ni/YSZ functional gradient anode supported solid oxide fuel cell. / Hao, Xiaoming; Han, Dongdong; Wang, Jiawei; Liu, Yajie; Rooney, David; Sun, Wang; Qiao, Jinshuo; Wang, Zhenhua; Sun, Kening.

In: International Journal of Hydrogen Energy, Vol. 40, No. 37, 05.10.2015, p. 12790-12797.

Research output: Contribution to journal › Article › peer-review

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AU - Hao, Xiaoming

AU - Han, Dongdong

AU - Wang, Jiawei

AU - Liu, Yajie

AU - Rooney, David

AU - Sun, Wang

AU - Qiao, Jinshuo

AU - Wang, Zhenhua

AU - Sun, Kening

PY - 2015/10/5

Y1 - 2015/10/5

N2 - The ability to directly utilize hydrocarbons and other renewable liquid fuels is one of the most important issues affecting the large scale deployment of solid oxide fuel cells (SOFCs). Herein we designed La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode (FGA) supported SOFCs, prepared with a co-tape casting method and sintered using the field assisted sintering technique (FAST). Through SEM observations, it was confirmed that the FGA structure was achieved and well maintained after the FAST process. Distortion and delamination which usually results after conventional sintering was successfully avoided. The La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs showed a maximum power density of 600mWcm-2 at 750°C, and was stable for 70h in CH4. No carbon deposition was detected using Raman spectroscopy. These results confirm the potential coke resistance of La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs.

AB - The ability to directly utilize hydrocarbons and other renewable liquid fuels is one of the most important issues affecting the large scale deployment of solid oxide fuel cells (SOFCs). Herein we designed La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode (FGA) supported SOFCs, prepared with a co-tape casting method and sintered using the field assisted sintering technique (FAST). Through SEM observations, it was confirmed that the FGA structure was achieved and well maintained after the FAST process. Distortion and delamination which usually results after conventional sintering was successfully avoided. The La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs showed a maximum power density of 600mWcm-2 at 750°C, and was stable for 70h in CH4. No carbon deposition was detected using Raman spectroscopy. These results confirm the potential coke resistance of La0.2Sr0.7TiO3-Ni/YSZ FGA supported SOFCs.

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KW - Lanthanum-doped strontium titanate

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EP - 12797

JO - International Journal of Hydrogen Energy

JF - International Journal of Hydrogen Energy

SN - 0360-3199

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Co-tape casting fabrication, field assistant sintering and evaluation of a coke resistant La0.2Sr0.7TiO3-Ni/YSZ functional gradient anode supported solid oxide fuel cell