Coproduction of Hydrogen and Carbon Filaments from Methane Decomposition over Fe/La2O3 Catalysts

Ahmed. Sadeq Al–Fatesh, Jehad Abu-Dahrieh, Ahmed Aidid Ibrahim, Anis Hamza Fakeeha, Wasim Ullah Khan

Research output: Contribution to journalArticle

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Abstract

Clean hydrogen production from catalytic methane decomposition has attracted the attention of many researchers as an alternative fuel source. In the present work, the catalytic decomposition of methane into hydrogen and carbon filaments on La2O3 doped Fe catalyst was investigated using 25% iron loading. The effect of reaction temperatures (500-750°C) over 25% Fe/La2O3 catalyst was studied. The catalysts before and after reaction were characterized by BET, XRD,H2-TPR, TGA, TPO, SEM and TEM. Stability studies of 25% Fe/ La2O3 at 750 °C for 360 min for one cycle and 5 regeneration cycles were carried out. The 25% Fe/ La2O3 catalyst showed high stability for the six cycles with no reduction in activity. Hence, iron supported over La2O3 catalyst is an efficient catalyst for hydrogen production from catalytic methane decomposition. SEM and TEM images exhibited formation of carbon filaments with various diameters and lengths.
Original languageEnglish
Pages (from-to)1104-1111
Number of pages8
JournalJournal of the chemical society of Pakistan
Volume38
Issue number6
Publication statusPublished - 01 Dec 2016

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Methane
Hydrogen
Carbon
Decomposition
Catalysts
Hydrogen production
Iron
Transmission electron microscopy
Scanning electron microscopy
Alternative fuels
Image processing

Cite this

Al–Fatesh, Ahmed. Sadeq ; Abu-Dahrieh, Jehad ; Ibrahim, Ahmed Aidid ; Fakeeha, Anis Hamza ; Khan, Wasim Ullah. / Coproduction of Hydrogen and Carbon Filaments from Methane Decomposition over Fe/La2O3 Catalysts. In: Journal of the chemical society of Pakistan. 2016 ; Vol. 38, No. 6. pp. 1104-1111.
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abstract = "Clean hydrogen production from catalytic methane decomposition has attracted the attention of many researchers as an alternative fuel source. In the present work, the catalytic decomposition of methane into hydrogen and carbon filaments on La2O3 doped Fe catalyst was investigated using 25{\%} iron loading. The effect of reaction temperatures (500-750°C) over 25{\%} Fe/La2O3 catalyst was studied. The catalysts before and after reaction were characterized by BET, XRD,H2-TPR, TGA, TPO, SEM and TEM. Stability studies of 25{\%} Fe/ La2O3 at 750 °C for 360 min for one cycle and 5 regeneration cycles were carried out. The 25{\%} Fe/ La2O3 catalyst showed high stability for the six cycles with no reduction in activity. Hence, iron supported over La2O3 catalyst is an efficient catalyst for hydrogen production from catalytic methane decomposition. SEM and TEM images exhibited formation of carbon filaments with various diameters and lengths.",
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Coproduction of Hydrogen and Carbon Filaments from Methane Decomposition over Fe/La2O3 Catalysts. / Al–Fatesh, Ahmed. Sadeq; Abu-Dahrieh, Jehad; Ibrahim, Ahmed Aidid; Fakeeha, Anis Hamza; Khan, Wasim Ullah.

In: Journal of the chemical society of Pakistan, Vol. 38, No. 6, 01.12.2016, p. 1104-1111.

Research output: Contribution to journalArticle

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AU - Al–Fatesh, Ahmed. Sadeq

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AU - Fakeeha, Anis Hamza

AU - Khan, Wasim Ullah

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AB - Clean hydrogen production from catalytic methane decomposition has attracted the attention of many researchers as an alternative fuel source. In the present work, the catalytic decomposition of methane into hydrogen and carbon filaments on La2O3 doped Fe catalyst was investigated using 25% iron loading. The effect of reaction temperatures (500-750°C) over 25% Fe/La2O3 catalyst was studied. The catalysts before and after reaction were characterized by BET, XRD,H2-TPR, TGA, TPO, SEM and TEM. Stability studies of 25% Fe/ La2O3 at 750 °C for 360 min for one cycle and 5 regeneration cycles were carried out. The 25% Fe/ La2O3 catalyst showed high stability for the six cycles with no reduction in activity. Hence, iron supported over La2O3 catalyst is an efficient catalyst for hydrogen production from catalytic methane decomposition. SEM and TEM images exhibited formation of carbon filaments with various diameters and lengths.

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