Expansion of pulse responses from temporal analysis of products (TAP) pulse responses for more accurate data analysis

Kevin Morgan, Alexandre Goguet, Christopher Hardacre, Evgenii V. Kondratenko, Colin McManus, Sergiy Shekhtman

Research output: Contribution to journalArticle

3 Citations (Scopus)

Abstract

TAP pulse responses are normally analysed using moments, which are integrals of the full TAP pulse response. However, in some cases the entire pulse response may not be recorded due to technical reasons, thereby compromising any data analysis due to moments generated from incomplete pulse responses. The current work discloses the development of a function which mathematically expands the tail of a TAP pulse response, so that the TAP data analysis can be accurately conducted. This newly developed analysis method has been applied to the oxidative dehydrogenation of ethane over Co–Cr–Sn–WOx/α-Al2O3 and Co–Cr–Sn–WOx/α-Al2O3 catalysts as a case study.
Original languageEnglish
Pages (from-to)3665-3671
Number of pages7
JournalCatalysis, Science & technology
Volume4
DOIs
Publication statusPublished - 01 Jul 2014

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