High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

D. Kraus; N. J. Hartley; S. Frydrych; A. K. Schuster; K. Rohatsch; M. Rödel; T. E. Cowan; S. Brown; E. Cunningham; T. Van Driel; L. B. Fletcher; E. Galtier; E. J. Gamboa; A. Laso Garcia; D. O. Gericke; E. Granados; P. A. Heimann; H. J. Lee; M. J. Macdonald; A. J. Mackinnon; E. E. McBride; I. Nam; P. Neumayer; A. Pak; A. Pelka; I. Prencipe; A. Ravasio; R. Redmer; A. M. Saunders; M. Schölmerich; M. Schörner; P. Sun; S. J. Turner; A. Zettl; R. W. Falcone; S. H. Glenzer; T. Döppner; J. Vorberger

doi:10.1063/1.5017908

High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

D. Kraus
, N. J. Hartley
, S. Frydrych
, A. K. Schuster
, K. Rohatsch
, M. Rödel
, T. E. Cowan
, S. Brown
, E. Cunningham
, T. Van Driel
, L. B. Fletcher
, E. Galtier
, E. J. Gamboa
, A. Laso Garcia
, D. O. Gericke
, E. Granados
, P. A. Heimann
, H. J. Lee
, M. J. Macdonald
, A. J. Mackinnon

E. E. McBride, I. Nam, P. Neumayer, A. Pak, A. Pelka, I. Prencipe, A. Ravasio, R. Redmer, A. M. Saunders, M. Schölmerich, M. Schörner, P. Sun, S. J. Turner, A. Zettl, R. W. Falcone, S. H. Glenzer, T. Döppner, J. Vorberger

Research output: Contribution to journal › Article › peer-review

36 Citations (Scopus)

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Abstract

Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

Original language	English
Article number	056313
Journal	Physics of Plasmas
Volume	25
Issue number	5
DOIs	https://doi.org/10.1063/1.5017908
Publication status	Published - 23 May 2018
Externally published	Yes

Bibliographical note

Funding Information:
This work was performed at the Matter at Extreme Conditions (MEC) instrument of LCLS, supported by the U.S. Department of Energy Office of Science, Fusion Energy Science under Contract No. SF00515. D.K., A.M.S., and R.W.F. acknowledge the support by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, and by the National Nuclear Security Administration under Award Nos. DE-FG52–10NA29649 and DE-NA0001859. D.K., N.J.H., A.K.S., and K.R. were supported by the Helmholtz Association under VH-NG-1141. N.J.H. was supported by Kakenhi Grant No. 16K17846. SLAC HED was supported by DOE Office of Science, Fusion Energy Science, under FWP 100182. S.F. was supported by German Bundesministerium fur Bildung und Forschung Project No. 05P15RDFA1. S.T. and A.Z. acknowledge support by the Air Force Office of Scientific Research under Award No. FA9550–14-1–0323 which provided for synthesis of low-density frameworks, and support from the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02–05-CH11231, within the sp2-Bonded Materials Program (KC2207) which provided for structural and chemical characterization. S.T. also received support from a National Science Foundation fellowship. R.R. acknowledges support from the DFG via the Research Unit FOR 2440. The work of A.P., S.F., and T.D. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52–07NA27344, and T.D. was supported by Laboratory Directed Research and Development (LDRD) Grant No. 18-ERD-033. R.W.F. acknowledges support of the University of California Center for Frontiers in High Energy Density Science.

Publisher Copyright:
© 2018 Author(s).

ASJC Scopus subject areas

Condensed Matter Physics

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10.1063/1.5017908Licence: CC BY

High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion
Copyright 2022 the authors. This is an open access article published under a Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
Final published version, 3.83 MBLicence: CC BY

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Kraus, D., Hartley, N. J., Frydrych, S., Schuster, A. K., Rohatsch, K., Rödel, M., Cowan, T. E., Brown, S., Cunningham, E., Van Driel, T., Fletcher, L. B., Galtier, E., Gamboa, E. J., Laso Garcia, A., Gericke, D. O., Granados, E., Heimann, P. A., Lee, H. J., Macdonald, M. J., ... Vorberger, J. (2018). High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion. Physics of Plasmas, 25(5), Article 056313. https://doi.org/10.1063/1.5017908

@article{cb2030f721b941f38049b4e7b47f8519,

title = "High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion",

abstract = "Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.",

author = "D. Kraus and Hartley, \{N. J.\} and S. Frydrych and Schuster, \{A. K.\} and K. Rohatsch and M. R{\"o}del and Cowan, \{T. E.\} and S. Brown and E. Cunningham and \{Van Driel\}, T. and Fletcher, \{L. B.\} and E. Galtier and Gamboa, \{E. J.\} and \{Laso Garcia\}, A. and Gericke, \{D. O.\} and E. Granados and Heimann, \{P. A.\} and Lee, \{H. J.\} and Macdonald, \{M. J.\} and Mackinnon, \{A. J.\} and McBride, \{E. E.\} and I. Nam and P. Neumayer and A. Pak and A. Pelka and I. Prencipe and A. Ravasio and R. Redmer and Saunders, \{A. M.\} and M. Sch{\"o}lmerich and M. Sch{\"o}rner and P. Sun and Turner, \{S. J.\} and A. Zettl and Falcone, \{R. W.\} and Glenzer, \{S. H.\} and T. D{\"o}ppner and J. Vorberger",

note = "Funding Information: This work was performed at the Matter at Extreme Conditions (MEC) instrument of LCLS, supported by the U.S. Department of Energy Office of Science, Fusion Energy Science under Contract No. SF00515. D.K., A.M.S., and R.W.F. acknowledge the support by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, and by the National Nuclear Security Administration under Award Nos. DE-FG52–10NA29649 and DE-NA0001859. D.K., N.J.H., A.K.S., and K.R. were supported by the Helmholtz Association under VH-NG-1141. N.J.H. was supported by Kakenhi Grant No. 16K17846. SLAC HED was supported by DOE Office of Science, Fusion Energy Science, under FWP 100182. S.F. was supported by German Bundesministerium fur Bildung und Forschung Project No. 05P15RDFA1. S.T. and A.Z. acknowledge support by the Air Force Office of Scientific Research under Award No. FA9550–14-1–0323 which provided for synthesis of low-density frameworks, and support from the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02–05-CH11231, within the sp2-Bonded Materials Program (KC2207) which provided for structural and chemical characterization. S.T. also received support from a National Science Foundation fellowship. R.R. acknowledges support from the DFG via the Research Unit FOR 2440. The work of A.P., S.F., and T.D. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52–07NA27344, and T.D. was supported by Laboratory Directed Research and Development (LDRD) Grant No. 18-ERD-033. R.W.F. acknowledges support of the University of California Center for Frontiers in High Energy Density Science. Publisher Copyright: {\textcopyright} 2018 Author(s).",

year = "2018",

month = may,

day = "23",

doi = "10.1063/1.5017908",

language = "English",

volume = "25",

journal = "Physics of Plasmas",

issn = "1070-664X",

publisher = "American Institute of Physics",

number = "5",

}

Kraus, D, Hartley, NJ, Frydrych, S, Schuster, AK, Rohatsch, K, Rödel, M, Cowan, TE, Brown, S, Cunningham, E, Van Driel, T, Fletcher, LB, Galtier, E, Gamboa, EJ, Laso Garcia, A, Gericke, DO, Granados, E, Heimann, PA, Lee, HJ, Macdonald, MJ, Mackinnon, AJ, McBride, EE, Nam, I, Neumayer, P, Pak, A, Pelka, A, Prencipe, I, Ravasio, A, Redmer, R, Saunders, AM, Schölmerich, M, Schörner, M, Sun, P, Turner, SJ, Zettl, A, Falcone, RW, Glenzer, SH, Döppner, T & Vorberger, J 2018, 'High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion', Physics of Plasmas, vol. 25, no. 5, 056313. https://doi.org/10.1063/1.5017908

TY - JOUR

T1 - High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

AU - Kraus, D.

AU - Hartley, N. J.

AU - Frydrych, S.

AU - Schuster, A. K.

AU - Rohatsch, K.

AU - Rödel, M.

AU - Cowan, T. E.

AU - Brown, S.

AU - Cunningham, E.

AU - Van Driel, T.

AU - Fletcher, L. B.

AU - Galtier, E.

AU - Gamboa, E. J.

AU - Laso Garcia, A.

AU - Gericke, D. O.

AU - Granados, E.

AU - Heimann, P. A.

AU - Lee, H. J.

AU - Macdonald, M. J.

AU - Mackinnon, A. J.

AU - McBride, E. E.

AU - Nam, I.

AU - Neumayer, P.

AU - Pak, A.

AU - Pelka, A.

AU - Prencipe, I.

AU - Ravasio, A.

AU - Redmer, R.

AU - Saunders, A. M.

AU - Schölmerich, M.

AU - Schörner, M.

AU - Sun, P.

AU - Turner, S. J.

AU - Zettl, A.

AU - Falcone, R. W.

AU - Glenzer, S. H.

AU - Döppner, T.

AU - Vorberger, J.

N1 - Funding Information: This work was performed at the Matter at Extreme Conditions (MEC) instrument of LCLS, supported by the U.S. Department of Energy Office of Science, Fusion Energy Science under Contract No. SF00515. D.K., A.M.S., and R.W.F. acknowledge the support by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, and by the National Nuclear Security Administration under Award Nos. DE-FG52–10NA29649 and DE-NA0001859. D.K., N.J.H., A.K.S., and K.R. were supported by the Helmholtz Association under VH-NG-1141. N.J.H. was supported by Kakenhi Grant No. 16K17846. SLAC HED was supported by DOE Office of Science, Fusion Energy Science, under FWP 100182. S.F. was supported by German Bundesministerium fur Bildung und Forschung Project No. 05P15RDFA1. S.T. and A.Z. acknowledge support by the Air Force Office of Scientific Research under Award No. FA9550–14-1–0323 which provided for synthesis of low-density frameworks, and support from the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02–05-CH11231, within the sp2-Bonded Materials Program (KC2207) which provided for structural and chemical characterization. S.T. also received support from a National Science Foundation fellowship. R.R. acknowledges support from the DFG via the Research Unit FOR 2440. The work of A.P., S.F., and T.D. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52–07NA27344, and T.D. was supported by Laboratory Directed Research and Development (LDRD) Grant No. 18-ERD-033. R.W.F. acknowledges support of the University of California Center for Frontiers in High Energy Density Science. Publisher Copyright: © 2018 Author(s).

PY - 2018/5/23

Y1 - 2018/5/23

N2 - Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

AB - Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

U2 - 10.1063/1.5017908

DO - 10.1063/1.5017908

M3 - Article

SN - 1070-664X

VL - 25

JO - Physics of Plasmas

JF - Physics of Plasmas

IS - 5

M1 - 056313

ER -

High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

Abstract

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