Observing time-dependent vibrational quantum dynamics in deuterium hydride molecular ions

J. McKenna, Chris Calvert, J. Wood, D.S. Murphy, I.C.E. Turcu, J.M. Smith, K.G. Ertel, O. Chekhlov, E.J. Divall, Jim McCann, Ian Williams

Research output: Contribution to journalArticlepeer-review

11 Citations (Scopus)

Abstract

Few-cycle laser pulses are used to "pump and probe" image the vibrational wavepacket dynamics of a HD+ molecular ion. The quantum dephasing and revival structure of the wavepacket are mapped experimentally with time-resolved photodissociation imaging. The motion of the molecule is simulated using a quantum-mechanical model predicting the observed structure. The coherence of the wavepacket is controlled by varying the duration of the intense laser pulses. By means of a Fourier transform analysis both the periodicity and relative population of the vibrational states of the excited molecular ion have been characterized.
Original languageEnglish
Pages (from-to)1127-1138
Number of pages12
JournalJournal of Modern Optics
Volume54
Issue number7
DOIs
Publication statusPublished - May 2007

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

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