Abstract
Understanding the mechanisms of proton energy deposition in matter and subsequent damage formation is fundamental to radiation science. Here we exploit the picosecond (10^{-12} s) resolution of laser-driven accelerators to track ultrafast solvation dynamics for electrons due to proton radiolysis in liquid water (H_{2}O). Comparing these results with modeling that assumes initial conditions similar to those found in photolysis reveals that solvation time due to protons is extended by >20 ps. Supported by magnetohydrodynamic theory this indicates a highly dynamic phase in the immediate aftermath of the proton interaction that is not accounted for in current models.
| Original language | English |
|---|---|
| Article number | 186001 |
| Number of pages | 7 |
| Journal | Physical Review Letters |
| Volume | 127 |
| Issue number | 18 |
| DOIs | |
| Publication status | Published - 29 Oct 2021 |
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