Structural investigations and magnetic properties of sol-gel Ni0.5Zn0.5Fe2O4 thin films for microwave heating

P.Z. Gao, Evgeny Rebrov, T.M.W.G.M. Verhoeven, J.C. Schouten, R. Kleismit, G. Kozlowski, J. Cetnar, Z. Turgut, G. Subramanyam

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Abstract

Nanocrystalline Ni0.5Zn0.5Fe2O4 thin films have been synthesized with various grain sizes by a sol-gel method on polycrystalline silicon substrates. The morphology, magnetic, and microwave absorption properties of the films calcined in the 673-1073 K range were studied with x-ray diffraction, scanning electron microscopy, x-ray photoelectron spectroscopy, atomic force microscopy, vibrating sample magnetometry, and evanescent microwave microscopy. All films were uniform without microcracks. Increasing the calcination temperature from 873 to 1073 K and time from 1 to 3 h resulted in an increase of the grain size from 12 to 27 nm. The saturation and remnant magnetization increased with increasing the grain size, while the coercivity demonstrated a maximum near a critical grain size of 21 nm due to the transition from monodomain to multidomain behavior. The complex permittivity of the Ni-Zn ferrite films was measured in the frequency range of 2-15 GHz. The heating behavior was studied in a multimode microwave cavity at 2.4 GHz. The highest microwave heating rate in the temperature range of 315-355 K was observed in the film close to the critical grain size.
Original languageEnglish
Article number044317
JournalJournal of Applied Physics
Volume107
Issue number4
DOIs
Publication statusPublished - 2010

ASJC Scopus subject areas

  • Physics and Astronomy(all)

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    Gao, P. Z., Rebrov, E., Verhoeven, T. M. W. G. M., Schouten, J. C., Kleismit, R., Kozlowski, G., Cetnar, J., Turgut, Z., & Subramanyam, G. (2010). Structural investigations and magnetic properties of sol-gel Ni0.5Zn0.5Fe2O4 thin films for microwave heating. Journal of Applied Physics, 107(4), [044317]. https://doi.org/10.1063/1.3309767