Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Christopher M.A. Parlett; Ayse Aydin; Lee J. Durndell; Lucia Frattini; Mark A. Isaacs; Adam F. Lee; Xiaotong Liu; Luca Olivi; Rima Trofimovaite; Karen Wilson; Chunfei Wu

doi:10.1016/j.catcom.2016.12.021

Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Christopher M.A. Parlett^*, Ayse Aydin, Lee J. Durndell, Lucia Frattini, Mark A. Isaacs, Adam F. Lee, Xiaotong Liu, Luca Olivi, Rima Trofimovaite, Karen Wilson, Chunfei Wu

^*Corresponding author for this work

School of Chemistry and Chemical Engineering

Research output: Contribution to journal › Article › peer-review

54 Citations (Scopus)

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Abstract

Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

Original language	English
Pages (from-to)	76-79
Number of pages	4
Journal	Catalysis Communications
Volume	91
Early online date	21 Dec 2016
DOIs	https://doi.org/10.1016/j.catcom.2016.12.021
Publication status	Published - 05 Mar 2017

Keywords

Ethanol steam reforming
Hydrogen production
Mesoporous materials
Nanoparticles
Nickel

ASJC Scopus subject areas

Catalysis
General Chemistry
Process Chemistry and Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1016/j.catcom.2016.12.021Licence: Unspecified

Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming
©2017 Elsevier. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
Accepted author manuscript, 714 KBLicence: CC BY-NC-ND

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title = "Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming",

abstract = "Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.",

keywords = "Ethanol steam reforming, Hydrogen production, Mesoporous materials, Nanoparticles, Nickel",

author = "Parlett, {Christopher M.A.} and Ayse Aydin and Durndell, {Lee J.} and Lucia Frattini and Isaacs, {Mark A.} and Lee, {Adam F.} and Xiaotong Liu and Luca Olivi and Rima Trofimovaite and Karen Wilson and Chunfei Wu",

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doi = "10.1016/j.catcom.2016.12.021",

language = "English",

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journal = "Catalysis Communications",

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AU - Parlett, Christopher M.A.

AU - Aydin, Ayse

AU - Durndell, Lee J.

AU - Frattini, Lucia

AU - Isaacs, Mark A.

AU - Lee, Adam F.

AU - Liu, Xiaotong

AU - Olivi, Luca

AU - Trofimovaite, Rima

AU - Wilson, Karen

AU - Wu, Chunfei

PY - 2017/3/5

Y1 - 2017/3/5

N2 - Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

AB - Mesoporous silica supported Ni nanoparticles have been investigated for hydrogen production from ethanol steam reforming. Ethanol reforming is structure-sensitive over Ni, and also dependent on support mesostructure; three-dimensional KIT-6 possessing interconnected mesopores offers superior metal dispersion, steam reforming activity, and on-stream stability against deactivation compared with a two-dimensional SBA-15 support.

KW - Ethanol steam reforming

KW - Hydrogen production

KW - Mesoporous materials

KW - Nanoparticles

KW - Nickel

UR - http://www.scopus.com/inward/record.url?scp=85007565840&partnerID=8YFLogxK

U2 - 10.1016/j.catcom.2016.12.021

DO - 10.1016/j.catcom.2016.12.021

M3 - Article

AN - SCOPUS:85007565840

SN - 1566-7367

VL - 91

SP - 76

EP - 79

JO - Catalysis Communications

JF - Catalysis Communications

ER -

Tailored mesoporous silica supports for Ni catalysed hydrogen production from ethanol steam reforming

Abstract

Keywords

ASJC Scopus subject areas

UN SDGs

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